Multiresonant Membrane Metasurfaces for Multifunctional Molecular Absorption Sensing and Real Time Biochemical Tracking
Quanlong Yang, Yapeng Dou, Dongyang Wang, Yihua Zhong, Fei Li, Jiajun He, Ying Zhang, Quan Xu 等 12 位
Central South University University of Southampton Yunnan Normal University Tianjin University
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摘要与影响
Label‐free identification and real time tracking of biochemical substances became critical for molecular diagnostics and chemical analysis, yet conventional resonant terahertz (THz) metasurface sensing relies on a single resonance, limiting spectral selectivity and dynamic capability. Here, we suggest multiresonant membrane metasurfaces and employ them for simultaneous static characteristic absorption detection and dynamic reaction monitoring within a single pixel. We consider a membrane metasurface supporting multiple quasi‐bound states in the continuum designed at target frequencies and enabling the tailoring of the field enhancement and frequency‐selective interaction with target analytes. As a proof‐of‐concept, we achieve label‐free detection of the characteristic absorption features of pefloxacin at 0.78 and 0.99 THz, and real time tracking of vitamin C oxidation and denaturation under ambient conditions. The kinetic profiles extracted from the THz amplitude evolution show excellent agreement with nonlinear reaction models (R 2 > 0.92), demonstrating quantitative biochemical tracking capabilities. Our results establish a versatile and scalable THz photonic platform that unifies static molecule identification and dynamic reaction monitoring, paving the way toward integrated on‐chip biochemical analytics and multifunctional metasurface sensors.
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材料 / 化学Metamaterials and Metasurfaces Applications
Terahertz technology and applications · Plasmonic and Surface Plasmon Research
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