Electrocatalytic amine dehydrogenation as a green route to nitriles: precise construction of efficient catalysts and mechanism

characterization, theoretical calculations, and performance evaluation, we further identify key future research directions, including multi-scale optimization of catalytic systems, electrolyzer design, and techno-economic analysis. This review aims to offer theoretical insights and practical guidance for the development of efficient, stable, and scalable electrocatalytic systems for green nitrile synthesis.