Symmetry Classification of Altermagnetism and Emergence of Type-IV Magnetism in Two Dimensions
Mu Tian, Chaoxi Cui, Zeying Zhang, Jingyi Duan, Wanxiang Feng, Run‐Wu Zhang
Beijing Institute of Technology Beijing University of Chemical Technology
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摘要与影响
Two-dimensional (2D) magnetism, particularly 2D altermagnetism (AM), has attracted considerable interest due to its exceptional physical properties and broad application potential. However, the classification of AM undergoes a fundamental paradigm shift when transitioning from three-dimensional (3D) to 2D symmetry-enforced fully compensated collinear magnetism-a shift that has remained largely overlooked. Here, by extending unconventional magnetism to 2D collinear systems, we identify the symmetry conditions and electronic band characteristics of a distinct magnetic phase: type-IV magnetism. This new class lies beyond the established descriptions of ferromagnetism, conventional antiferromagnetism, and AM. Type-IV magnetism supports the successive emergence of both nonrelativistic spin-degenerate and relativistic spin-splitting phenomena, belonging strictly to neither conventional antiferromagnetism nor standard AM. We further establish a universal symmetry classification framework for 2D type-IV magnets via a mapping from the collinear spin layer group to the magnetic layer group. Monolayer MgCr_{2}O_{4} and monolayer BaMn_{2}Ch_{3} (Ch=Se, Te) are showcased as representative materials, exhibiting gate-tunable reversible spin textures and the quantum electric Hall effect, respectively. Our Letter underscores the rich functional prospects of type-IV magnets, offering a new route toward spin manipulation and anomalous transport that promises innovative designs for high-performance spintronic devices.
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物理Magnetic properties of thin films
Advanced Condensed Matter Physics · Topological Materials and Phenomena
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